When talking to children, don't ask or expect them to smile well on cue.
Tell them to wet their lips and close them a bit.
Then take one shot and tell them to fart.
When they laugh take more shots.
These fake smiles are just torture.
Slow down, take a step back and work on getting better composition.
Both pictures are badly tilted and not well placed in the frame.
In the first, they are way too low in the frame and chopped off but there is a lot of space above them; it looks like a framing mistake.
The second one is shot out in the direct sun, badly tilted, there are burnt out areas on her face and the background is terribly annoying and ugly and there is so much of it.
Don't convert to B&W to try and save it, toss it.